Wei-Hao ChiuAcademic Profile

International Journal Publication

Effects of mesoscopic poly (3, 4-ethylenedioxythiophene) films as counter electrodes for dye-sensitized solar cells

Author affiliations and roles
  1. aIndustrial Technology Research Institute
  2. bNational Yang Ming Chiao Tung University
  3. cNational Taiwan University
  4. dCentral Electrochemical Research Institute
  • *Corresponding authors: Lee, Kun-Mu, Ho, Kuo-Chuan.

Thin Solid Films, 518, 1716–1721 (2010).

Research topic: Dye-Sensitized Solar Cells

Abstract

Counter electrode coated with chemically polymerized poly(3,4-ethylenedioxythiophene) (PEDOT) in a dye-sensitized solar cell (DSSC) was studied. The surface morphology and the nature of I(-)/I(3)(-) redox reaction based on PEDOT film were investigated using Atomic Force Microscopy and Cyclic Voltammetry, respectively. The performance of the DSSCs containing the PEDOT coated electrode was compared with sputtered-Pt electrode. We found that the root mean square roughness decreases and conductivity increases as the molar ratio of imidazole (Im)/EDOT in the PEDOT film increases. The DSSC containing the PEDOT coated on fluorine doped tin oxide glass with Im/EDOT molar ratio of 2.0, showed a conversion efficiency of 7.44% compared to that with sputtered-Pt electrode (7.77%). The high photocurrents were attributed to the large effective Surface area of the electrode material resulting in good catalytic properties for T(3) reduction. Therefore, the incorporation of a multi-walled carbon nanotube (MWCNT) in the PEDOT film, coated on various substrates was also investigated. The DSSC containing the PEDOT films with 0.6 wt.% of MWCNT on stainless steel as counter electrode had the best cell performance of 8.08% with short-circuit current density, open-circuit voltage and fill factor of 17.00 mA cm(-2), 720 mV and 0.66, respectively. (C) 2009 Elsevier B.V. All rights reserved.

Keywords

Conducting polymerDye-sensitized solar cellsCounter electrodePoly(3,4-ethylenedioxythiophene)Carbon nanotubes
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